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Journal Articles

Neutron transmission CB-KID imager using samples placed at room temperature

Ishida, Takekazu*; Vu, TheDang*; Shishido, Hiroaki*; Aizawa, Kazuya; Oku, Takayuki; Oikawa, Kenichi; Harada, Masahide; Kojima, Kenji M*; Miyajima, Shigeyuki*; Koyama, Tomio*; et al.

Journal of Low Temperature Physics, 214(3-4), p.152 - 157, 2024/02

 Times Cited Count:0 Percentile:0.02(Physics, Applied)

Journal Articles

Observation of gamma rays up to 320 TeV from the middle-aged TeV pulsar wind nebula HESS J1849-000

Amenomori, Michihiro*; Tsuchiya, Harufumi; Tibet AS$$gamma$$ Collaboration*; 116 of others*

Astrophysical Journal, 954(2), p.200_1 - 200_7, 2023/09

 Times Cited Count:1 Percentile:50.15(Astronomy & Astrophysics)

Journal Articles

Orientation mapping of YbSn$$_{3}$$ single crystals based on Bragg-dip analysis using a delay-line superconducting sensor

Shishido, Hiroaki*; Vu, TheDang*; Aizawa, Kazuya; Kojima, Kenji M*; Koyama, Tomio*; Oikawa, Kenichi; Harada, Masahide; Oku, Takayuki; Soyama, Kazuhiko; Miyajima, Shigeyuki*; et al.

Journal of Applied Crystallography, 56(4), p.1108 - 1113, 2023/08

 Times Cited Count:0 Percentile:0.02(Chemistry, Multidisciplinary)

Journal Articles

Radioisotope identification algorithm using deep artificial neural network for supporting nuclear detection and first response on nuclear security incidents

Kimura, Yoshiki; Tsuchiya, Kenichi*

Radioisotopes, 72(2), p.121 - 139, 2023/07

Rapid and precise radioisotope identification in the scene of nuclear detection and nuclear security incidents is one of the challenging issues for the prompt response on the detection alarm or the incidents. A radioisotope identification algorithm using a deep artificial neural network model applicable to handheld gamma-ray detectors has been proposed in the present paper. The proposed algorithm automatically identifies gamma-emitting radioisotopes based on the count contribution ratio (CCR) from each of them estimated by the deep artificial neural network model trained by simulated gamma-ray spectra. The automated radioisotope identification algorithm can support first responders of nuclear detection and nuclear security incidents without sufficient experience and knowledge in radiation measurement. The authors tested the performance of the proposed algorithm using two different types of deep artificial neural network models in application to handheld detectors having high or low energy resolution. The proposed algorithm showed high performance in identifying artificial radioisotopes for actually measured gamma-ray spectra. It was also confirmed that the algorithm is applicable to identifying $$^{235}$$U and automated uranium categorization by analyzing estimated CCRs by the deep artificial neural network models. The authors also com-pared the performance of the proposed algorithm with a conventional radioisotope identification method and discussed promising ways to improve the performance of the algorithm using the deep artificial neural network.

JAEA Reports

Development of wide range monitor for HTTR; Improvement for heat resistance performance against heat cycle

Kozawa, Takayuki; Suganuma, Takuro; Homma, Fumitaka; Higashimura, Keisuke*; Ukai, Takayuki*; Saito, Kenji

JAEA-Technology 2023-007, 24 Pages, 2023/06

JAEA-Technology-2023-007.pdf:2.24MB

To improve the reliability of the HTTR wide range monitor in a high-temperature environment, structural changes of the wide range monitor were investigated. It was clear that the structure for directly joins of the MI cable core wire and metal tube instead of the joins with lead wire is the most reliable method with shortest way. From a result of the thermal cycle tests and high temperature endurance tests for a mock-up connecting this connection parts, it was clear that the soundness of the connection part was maintained under the usage conditions of the HTTR.

Journal Articles

Shield-free directional gamma-ray detector using small-angle Compton scattering

Kitayama, Yoshiharu

Gamma Ray Imaging; Technology and Applications, p.165 - 179, 2023/00

A gamma-ray imager is a powerful tool for visualizing the distribution of radioactive materials. Recently, it has been applied to the decommissioning site of the Fukushima Daiichi Nuclear Power Station. At the decommissioning site, an imager compact, lightweight, and capable of quantitative evaluation of radioactivity is demanded. The Gamma-ray Imager using Small-Angle Scattering (GISAS) was proposed as a gamma-ray imager that meets all these requirements. GISAS consists of several shield-free directional gamma-ray detectors that detect only small-angle Compton scattering. Simulations and experiments verified the feasibility of the shield-free directional gamma-ray detectors. The shield-free directional gamma-ray detector consists of a scatterer that detects small-angle Compton scattering and an absorber that detects the scattered gamma rays. By setting an appropriate energy window for each detector, only scattering events that can be considered almost straightforward are detected. Through simulations and experiments, we have confirmed that using a silicon drift detector as the scatterer and a Gd3Al2Ga3O12 scintillator as the absorber, we can detect only small-angle Compton scattering events and obtain directionality for 662 keV gamma rays.

Journal Articles

Application of high-energy-resolution X-ray absorption spectroscopy at the U L$$_{3}$$-edge to assess the U(V) electronic structure in FeUO$$_{4}$$

Yomogida, Takumi; Akiyama, Daisuke*; Ouchi, Kazuki; Kumagai, Yuta; Higashi, Kotaro*; Kitatsuji, Yoshihiro; Kirishima, Akira*; Kawamura, Naomi*; Takahashi, Yoshio*

Inorganic Chemistry, 61(50), p.20206 - 20210, 2022/12

 Times Cited Count:2 Percentile:36.89(Chemistry, Inorganic & Nuclear)

FeUO$$_{4}$$ was studied to clarify the electronic structure of U(V) in a metal monouranate compound. We obtained the peak splitting of HERFD-XANES spectra utilizing high-energy-resolution fluorescence detection-X-ray absorption near edge structure (HERFD-XANES) spectroscopy at the U L$$_{3}$$-edge, which is a novel technique in the U(V) compounds. Theoretical calculations revealed that the peak splitting was caused by splitting the 6d orbital of U(V). Such distinctive electronic states are of major interest to researchers and engineers working in various fields, from fundamental physics to the nuclear industry and environmental sciences for actinide elements.

Journal Articles

Evaluation of detector performances of new thin position-sensitive scintillation detectors for SENJU diffractometer

Nakamura, Tatsuya; To, Kentaro; Koizumi, Tomokatsu; Kiyanagi, Ryoji; Ohara, Takashi; Ebine, Masumi; Sakasai, Kaoru

Proceedings of 2022 IEEE Nuclear Science Symposium, Medical Imaging Conference and Room Temperature Semiconductor Detector Conference (2022 IEEE NSS MIC RTSD) (Internet), 2 Pages, 2022/11

A new thin position-sensitive scintillation neutron detectors have been developed to replace present scintillation detectors in SENJU diffractometer at J-PARC MLF. The SENJU diffractometer originally composed of 37 position-sensitive detectors, where each detector has neutron sensitive area of 256 $$times$$ 256 mm with a pixel size of 4 $$times$$ 4 mm. To renew some original detectors the new detectors have been developed based on ZnS scintillator and wavelength-shifting fibers technology. The developed replacement detectors were designed with a thin thickness of 12 cm, which is 40% of the original detector. The new detectors have also improved detector performances to the original ones in terms of detection efficiency ($$sim$$60% for 2-A neutrons) and count uniformity (5-8%). The produced six detector modules have been implemented to the beamline after checking their detector performances in the lab.

Journal Articles

Absolute quantification of $$^{137}$$Cs activity in spent nuclear fuel with calculated detector response function

Sato, Shunsuke*; Nauchi, Yasushi*; Hayakawa, Takehito*; Kimura, Yasuhiko; Kashima, Takao*; Futakami, Kazuhiro*; Suyama, Kenya

Journal of Nuclear Science and Technology, 60(6), p.615 - 623, 2022/06

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

A new non-destructive method for evaluating $$^{137}$$Cs activity in spent nuclear fuels was proposed and experimentally demonstrated for physical measurements in burnup credit implementation. $$^{137}$$Cs activities were quantified using gamma ray measurements and numerical detector response simulations without reference fuels, in which $$^{137}$$Cs activities are well known. Fuel samples were obtained from a lead use assembly (LUA) irradiated in a commercial pressurized water reactor (PWR) up to 53 GWd/t. Gamma rays emitted from the samples were measured using a bismuth germinate (BGO) scintillation detector through a collimator attached to a hot cell. The detection efficiency of gamma rays with the detector was calculated using the PHITS particle transport calculation code considering the measurement geometry. The relative activities of $$^{134}$$Cs, $$^{137}$$Cs, and $$^{154}$$Eu in the sample were measured with a high-purity germanium (HPGe) detector for more accurate simulations of the detector response for the samples. The absolute efficiency of the detector was calibrated by measuring a standard gamma ray source in another geometry. $$^{137}$$Cs activity in the fuel samples was quantified using the measured count rate and detection efficiency. The quantified $$^{137}$$Cs activities agreed well with those estimated using the MVP-BURN depletion calculation code.

Journal Articles

Computed tomography neutron detector system to observe power distribution in a core with long neutron flight path

Fukaya, Yuji; Okita, Shoichiro; Nakagawa, Shigeaki; Goto, Minoru; Ohashi, Hirofumi

Annals of Nuclear Energy, 168, p.108911_1 - 108911_7, 2022/04

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

A power distribution monitoring system by using a moving detector for a core with a long neutron flight path has been proposed. High Temperature Gas-cooled Reactor (HTGR) and Fast Reactor (FR) has a long neutron flight path and the neutrons reach to detector far from fuel assembly in the center of the core unlike Light Water Reactor (LWR). By using the feature, power distribution can be observed with a few detectors by moving the detector and computed tomography technology similar to X-ray Computed Tomography (CT). For a small-sized core, the power distribution can be evaluated only by an ex-core neutron detector. For a large-sized core with inner detectors, the power distribution can be observed with a small number of in-core detectors even if the deployment is limited due to material integrity conditions such as temperature environment. The feasibility is numerically confirmed by simulations of the HTGR core and its detector response. It is expected to observe the power distribution in the core of HTGR and FR, which is difficult continuously to deploy in-core detectors because of high temperature and/or high irradiation damage.

JAEA Reports

Calculation code of output current for self-powered radiation detector; Algorithm construction and comparison of calculation results

Shibata, Hiroshi; Takeuchi, Tomoaki; Seki, Misaki; Shibata, Akira; Nakamura, Jinichi; Ide, Hiroshi

JAEA-Data/Code 2021-018, 42 Pages, 2022/03

JAEA-Data-Code-2021-018.pdf:2.78MB
JAEA-Data-Code-2021-018-appendix(CD-ROM).zip:0.15MB

Japan Materials Testing Reactor (JMTR) in Oarai Research and Development Institute of the Japan Atomic Energy Agency has been developing various reactor materials, irradiation techniques and instruments for more than 30 years. Among them, the development of self-powered neutron detectors (SPNDs) and gamma detectors (SPGDs) has been carried out, and several research results have been reported. However, most of the results are based on the design study of the detector development and the results of in-core irradiation tests and gamma irradiation tests using Cobalt-60. In this report, a numerical code is developed based on the paper "Neutron and Gamma-Ray Effects on Self-Powered In-Core Radiation Detectors" written by H.D. Warren and N.H. Shah in 1974, in order to theoretically evaluate the self-powered radiation detectors.

Journal Articles

Quantitation of trace lanthanide and actinide ions in radioactive samples by capillary electrophoresis-laser-induced fluorescence detection

Haraga, Tomoko; Saito, Shingo*

Bunseki Kagaku, 70(12), p.671 - 679, 2021/12

We developed highly sensitive capillary electrophoresis-laser-induced fluorescence detection methods for lanthanide (Ln) and actinide (An) ions with small sample volume and low emission of waste, by which the radiation risk can be minimized. Specifically, determination of Nd ion in spent nuclear fuel, effective separation between Am and Cm ion, and specific detection of UO$$_{2}$$$$^{2+}$$ in real radioactive samples were achieved by molecular design of fluorescence probes composed of an aminocarboxylate chelating moiety, a fluorophore and a spacer, and unique separation mode based on dynamic ternary complexation. We found that there are appropriate combination of probe and ternary complexation for detection and separation of each Ln and An ions. For example, acyclic and macrocyclic hexadentate is suitable for Ln$$^{3+}$$, Am$$^{3+}$$ and Cm$$^{3+}$$, and planer tetradentate with $$pi$$ electron system is specific for UO$$_{2}$$$$^{2+}$$, with ppt-sub ppt level detection.

Journal Articles

High spatial resolution neutron transmission imaging using a superconducting two-dimensional detector

Shishido, Hiroaki*; Nishimura, Kazuma*; Vu, TheDang*; Aizawa, Kazuya; Kojima, Kenji M*; Koyama, Tomio*; Oikawa, Kenichi; Harada, Masahide; Oku, Takayuki; Soyama, Kazuhiko; et al.

IEEE Transactions on Applied Superconductivity, 31(9), p.2400505_1 - 2400505_5, 2021/12

 Times Cited Count:0 Percentile:0(Engineering, Electrical & Electronic)

In this study, we employed a superconducting detector, current-biased kinetic-inductance detector (CB-KID) for neutron imaging using a pulsed neutron source. We employed the delay-line method, and high spatial resolution imaging with only four reading channels was achieved. We also performed wavelength-resolved neutron imaging by the time-of-flight method. We obtained the neutron transmission images of a Gd-Al alloy sample, inside which single crystals of GdAl$$_{3}$$ were grown, using the delay-line CB-KID. Single crystals were well imaged, in both shapes and distributions, throughout the Al-Gd alloy. We identified Gd nuclei via neutron transmissions that exhibited characteristic suppression above the neutron wavelength of 0.03 nm. In addition, the $$_{155}$$Gd resonance dip, a dip structure of the transmission caused by the nuclear reaction between an isotope and neutrons, was observed even when the number of events was summed over a limited area of 15 $$mu$$m $$times$$ 12 $$mu$$m. Gd selective imaging was performed using the resonance dip of $$_{155}$$Gd, and it showed clear Gd distribution even with a limited neutron wavelength range of 1 pm.

Journal Articles

Monitoring technique for detection of nuclear and radioactive materials on major public events

Mochimaru, Takanori*; Koizumi, Mitsuo; Takahashi, Tone; Hironaka, Kota; Kimura, Yoshiki; Sato, Yuki; Terasaka, Yuta; Yamanishi, Hirokuni*; Wakabayashi, Genichiro*

Dai-42-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2021/11

no abstracts in English

Journal Articles

Simulation study of a shield-free directional gamma-ray detector using Small-Angle Compton Scattering

Kitayama, Yoshiharu; Terasaka, Yuta; Sato, Yuki; Torii, Tatsuo

Journal of Nuclear Engineering and Radiation Science, 7(4), p.042006_1 - 042006_7, 2021/10

Journal Articles

Two-dimensional scintillation neutron detectors for the extension of SENJU diffractometer

Nakamura, Tatsuya; To, Kentaro; Koizumi, Tomokatsu; Kiyanagi, Ryoji; Ohara, Takashi; Ebine, Masumi; Sakasai, Kaoru

Proceedings of 2020 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2020), Vol.1, p.483 - 484, 2021/09

Two-dimensional neutron detectors were developed for the extension of SENJU time-of-flight Laue single crystal neutron diffractometer in J-PARC MLF. The detectors are to be installed at the additional detector bank for the SENJU instrument. The detector module is made based on ZnS scintillator and wavelength-shifting fiber technology, where each detector module maintains a neutron-sensitive area of 256$$times$$256 mm with a pixel size of 4$$times$$4 mm. To meet the tight space limitation in the instrument, the detector was designed as compact as possible. The detector has a depth of 170 mm, which is about 40% smaller than that of the original SENJU detector. All four produced detectors exhibited similar detector performances: detection efficiency 50-60% for 2-${AA}$ neutron, $$^{60}$$Co gamma-ray sensitivity 1$$times$$10$$^{-5}$$, count uniformity 3-6%.

Journal Articles

Gamma-ray observation of the Cygnus region in the 100-TeV energy region

Amenomori, Michihiro*; Tsuchiya, Harufumi; Tibet AS$$_{gamma}$$ Collaboration*; 111 of others*

Physical Review Letters, 127(3), p.031102_1 - 031102_6, 2021/07

 Times Cited Count:18 Percentile:87.51(Physics, Multidisciplinary)

Journal Articles

Potential PeVatron supernova remnant G106.3+2.7 seen in the highest-energy gamma rays

Amenomori, Michihiro*; Tsuchiya, Harufumi; Tibet AS$$_{gamma}$$ Collaboration*; 93 of others*

Nature Astronomy (Internet), 5(5), p.460 - 464, 2021/05

 Times Cited Count:64 Percentile:98.97(Astronomy & Astrophysics)

Journal Articles

First detection of sub-PeV diffuse gamma rays from the galactic disk; Evidence for ubiquitous galactic cosmic rays beyond PeV energies

Amenomori, Michihiro*; Tsuchiya, Harufumi; Tibet AS$$_{gamma}$$ Collaboration*; 93 of others*

Physical Review Letters, 126(14), p.141101_1 - 141101_7, 2021/04

 Times Cited Count:112 Percentile:99.57(Physics, Multidisciplinary)

Journal Articles

Photonuclear reactions in lightning, 1; Verification and modeling of reaction and propagation processes

Wada, Yuki*; Enoto, Teruaki*; Nakazawa, Kazuhiro*; Odaka, Hirokazu*; Furuta, Yoshihiro; Tsuchiya, Harufumi

Journal of Geophysical Research; Atmospheres, 125(20), p.e2020JD033193_1 - e2020JD033193_17, 2020/10

 Times Cited Count:3 Percentile:15.82(Meteorology & Atmospheric Sciences)

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